The singer was married to Harry's son Jamie for almost 20 years, and he was extremely fond of the former Eternal star.
In his 1998 autobiography, Harry, 71, opened up about his relationship with Jamie's then-wife, 44, who is the mother of his two grandsons.
Harry, 71, revealed he always saw Louise as a "nice" and "caring" person and struggled to understand her role as a saucy pop star.
He wrote: "Louise… is the most down-to-earth girl you could hope to meet.
"She may be a pop-star temptress to the youngsters who read those laddish magazine but to me she's just a lovely girl who's married to my youngest son.
"Louise… is the least showbizzy person you could imagine.
"She's so quiet and shy away from the spotlight that I can't believe she has the front to go live on stage in front of thousands of people.
"I see her in those glamorous videos for her latest record and find it impossible to reconcile the sexy image I see on screen with the Louise who comes to my home with Jamie for Sunday dinner."
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Louise and Jamie split last year, but Harry was always big supporter of their marriage and said they made a "lovely couple".
He added: "Jamie and her make a lovely couple, so Sandra and I were thrilled when the two of them got married. Jamie couldn't have met a nicer girl. She's a very caring person"
The couple married in Bermuda in July 1998 and went on to have two sons together.
They split last year and their divorce was finalised in late 2017.
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